Interaction of SiC with Al2O3−(t + m)ZrO2(Y2O3) Oxide Composition

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We employed contact alloying in the range 1000–1860°С to study the reaction specifics between SiC and Al2O3−(t + m)ZrO2(Y2O3) oxide composition. Real-time experiments with photographic recording of the changing size and shape of the Al2O3−(t + m)ZrO2(Y2O3) sample on a SiC ceramic substrate showed that Al2O3−(t + m)ZrO2(Y2O3) compositions react with the silicon carbide substrate in the range 1720–1860°С to melt and penetrate into (impregnate) the substrate. X-ray powder diffraction patterns were measured for samples taken from the contact area of the oxide composition with SiC directly on the substrate and in a chipped-off <1-mm-deep near-surface layer. ZrС, Al2Y4O9, and Al3.21Si0.47 were formed in the contact area via redox reactions involving oxide melt, in addition to 6H-SiC, Si and Al2O3, t-ZrO2 phases, which are the initial components of the substrate and oxide composition, respectively.

作者简介

A. Ivannikov

Baikov Institute of Metallurgy and Materials Science, Russian Academy of Sciences

Email: frolovamarianna@bk.ru
119334, Moscow, Russia

M. Mel’nikov

Baikov Institute of Metallurgy and Materials Science, Russian Academy of Sciences; Mendeleev Russian University of Chemical Technologies

Email: frolovamarianna@bk.ru
119334, Moscow, Russia; 125048, Moscow, Russia

Yu. Kargin

Baikov Institute of Metallurgy and Materials Science, Russian Academy of Sciences

Email: frolovamarianna@bk.ru
119334, Moscow, Russia

M. Frolova

Baikov Institute of Metallurgy and Materials Science, Russian Academy of Sciences

Email: frolovamarianna@bk.ru
119334, Moscow, Russia

A. Lysenkov

Baikov Institute of Metallurgy and Materials Science, Russian Academy of Sciences

Email: frolovamarianna@bk.ru
119334, Moscow, Russia

S. Perevislov

Grebenshchikov Institute of Silicate Chemistry, Russian Academy of Sciences

Email: frolovamarianna@bk.ru
199034, St. Petersburg, Russia

N. Petrakova

Baikov Institute of Metallurgy and Materials Science, Russian Academy of Sciences

Email: frolovamarianna@bk.ru
119334, Moscow, Russia

K. Kim

Baikov Institute of Metallurgy and Materials Science, Russian Academy of Sciences

Email: frolovamarianna@bk.ru
119334, Moscow, Russia

M. Sevost’yanov

Baikov Institute of Metallurgy and Materials Science, Russian Academy of Sciences

编辑信件的主要联系方式.
Email: frolovamarianna@bk.ru
119334, Moscow, Russia

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版权所有 © М.Г. Фролова, А.С. Лысенков, С.Н. Перевислов, Н.В. Петракова, К.А. Ким, М.А. Севостьянов, А.Ю. Иванников, М.Д. Мельников, Ю.Ф. Каргин, 2023